The Good Shepherd (2006)
Matt Damon is at his most blank-faced in this tale detailing the founding of the Central Intelligence Agency. He's literally a cipher. His wife doesn't know him, his odd-faced son doesn't know him, and we don't know him. Damon gives nothing awayhis face as stone-cold immobile here as it is in the Bourne films, which pretty much means he's perfect for the role.
Directed by Robert De Niro, Shepherd has an all-star cast of gravelly-voiced, suspicious-looking men: Alec Baldwin, Joe Pesci, William Hurt, John Turturro, and De Niro himself. The movie is swaddled in hushed-tone secret telling, and everyone's face looks drawn tight with the sheer effort of keeping mum. Slow-moving and grim, The Good Shepherd makes the list through sheer definitiveness.
From the TIME archives, Richard Corliss' Top Ten Films of 2006.

For the Post Office: Snow, Rain and Now Gloom of Recession
Travel: Energy Chews to Fight Jet Lag
Bride Wars: One Bride Too Many
Alfred Shaheen: Pioneer of the Hawaiian Shirt
Introducing MNN, the New 'Green CNN'
The Milky Way: Bigger, Faster, Better Understood
Video: Financial News in Old Fez
Top 10 Contested Officeholders
Q&A: Lessons from the Great Depression
Golfer's Ear: Can Big Drives Hurt Your Hearing?